THERMAL SCIENCE
International Scientific Journal
EXPERIMENTAL STUDIES ON THE VISCOSITY OF FE NANOPARTICLES DISPERSED IN ETHYLENE GLYCOL AND WATER MIXTURE
ABSTRACT
In this paper, experimental studies are conducted in order to measure the viscosity of Fe nanoparticles dispersed in various weight concentration (25/75%, 45/55% and 55/45%) of ethylene glycol and water (EG-water) mixture. The experimental measurements are performed at various volume concentrations up to 2% and temperature ranging from 10°C to 60°C. The experimental results disclose that the viscosity of nanofluids increases with increase in Fe particle volume fraction, and decreases with increase in temperature. Maximum enhancement in viscosity of nanofluids is 2.14 times for 55/45% EG-water based nanofluid at 2% volume concentration compared to the base fluid. Moreover, some comparisons between experimental results and theoretical models are drawn. It is also observed that the prior theoretical models do not estimate the viscosity of nanofluid accurately. Finally, a new empirical correlation is proposed to predict the viscosity of nanofluids as a function of volume concentration, temperature, and the viscosity of base fluid.
KEYWORDS
PAPER SUBMITTED: 2014-03-08
PAPER REVISED: 2015-01-16
PAPER ACCEPTED: 2015-03-08
PUBLISHED ONLINE: 2015-03-08
THERMAL SCIENCE YEAR
2016, VOLUME
20, ISSUE
Issue 5, PAGES [1661 - 1670]
- Eiyad, A.N., Effects of Variable Viscosity and Thermal Conductivity of CuO-Water Nanofluid on Heat Transfer Enhancement in Natural Convection: Mathematical Model and Simulation, J. Heat Transfer (ASME), 132 (2010), 5, pp. 052401(9 pages).
- Choi, S.U.S., Eastman, J.A., Enhancing Thermal Conductivity of Fluids with Nanoparticles, International mechanical engineering congress and exhibition, San Francisco, CA, United States, pp. 12-17.
- Daungthongsuk, W., Wongwises, S., A Critical Review of Convective Heat Transfer Nanofluids, Renewable Sustainable Energy Rev., 11 (2007), 5, pp. 797-817.
- Namburu, P.K., Kulkarni D.P., Misra, D., Das, D.K., Viscosity of copper oxide nanoparticles dispersed in ethylene glycol and water mixture, Exp. Therm. Fluid Sci., 32 (2007), pp. 397-402.
- Lin CY., Wang JC., Chen TC., Analysis of suspension and heat transfer characteristics of Al2O3 nanofluids prepared through ultrasonic vibration. Appl. Energy, 88 (2011), 12, pp. 4527-33.
- Wang, X.Q., Mujumdar, A.S., Heat transfer characteristics of nanofluids: a review, Int. J. Therm. Sci., 46 (2007), pp. 1-19.
- Velagapudi, V., Rama, K.K, Chandra, A.K.S., Empirical correlation to predict thermophysical and heat transfer characteristics of nanofluids, Therm. Sci., 12 (2008), 2, pp. 27-37.
- Murugesan, C., Sivan, S., Limits for thermal conductivity of nanofluids, Therm. Sci., 14 (2010), 1, pp. 65-71.
- Shanthi, R., Anandan, S.S., Ramalimgam, V., Heat transfer enhancement using nanofluids an overview, Therm. Sci., 16 (2012), 2, pp. 423-444.
- Risi, A.D., Marco, M., Gianpiero, C., Domenico, L., High efficiency nanofluid cooling system for wind turbines, Therm. Sci., 18 (2014), 2, pp. 543-554.
- Viota, J.L., Gonza´ lez-Caballero, F., Dura´ n, J.D.G., Delgado, A.V., Study of the colloidal stability of concentrated bimodal magnetic fluids, J. Colloid Interface Sci., 309 (2007), 1, pp. 135-139.
- Li, Q., Xuan, Y., Experimental investigation on heat transfer characteristics of magnetic fluid flow around a fine wire under the influence of an external magnetic field, Exp. Therm. Fluid Sci., 33 (2009), 4, pp. 591-596.
- Dobson, J., Magnetic nanoparticles for drug delivery, Drug develop Res, 67 (2006), 1, pp. 55-60.
- Kim, E.H., Lee, H.S., Kwak, B.K., Kim, B.K., Synthesis of ferrofluid with magnetic nanoparticles by sonochemical method for MRI contrast agent, J. Magn. Magn. Mater. 289 (2005), pp. 328-330.
- Pak BC., Cho YI., Hydrodynamic and heat transfer study of dispersed fluids with submicron metallic oxide particles, Exp. Heat Transfer, 11 (1998), pp. 151-70.
- Masuda H., Ebata A., Teramae K., Hishinuma N., Alteration of thermal conductivity and viscosity of liquid by dispersing ultra-fine particles (dispersion of - Al2O3, SiO2 and TiO2 ultra-fine particles). Netsu Bussei, 4 (1993), pp. 227-33.
- He, Y., Jin, Y., Chen, H., Ding, Y., Cang, D., Lu, H., Heat transfer and flow behavior of aqueous suspensions of TiO2 nanoparticles (Nanofluids) flowing upward through a vertical pipe, Int. J. Heat Mass Transfer, 50 (2007), pp. 2272-2281.
- Nguyen CT., Desgranges F., Roy G., Galanis N., Mare T., Boucher S., Temperature and particle-size dependent viscosity data for water-based nanofluids - Hysteresis phenomenon. Int. J. Heat Fluid Flow, 28 (2007), pp. 1492-506.
- Lee JH., Hwang KS., Jang SP., Lee BH., Kim JH., Choi SUS., Effective viscosities and thermal conductivities of aqueous nanofluids containing low volume concentrations of Al2O3 nanoparticles, Int. J. Heat. Mass. Transfer, 51 (2008), pp. 2651-2656.
- Murshed SMS., Leong KC., Yang C., Investigations of thermal conductivity and viscosity of nanofluids, Int. J. Therm. Sci. 47 (2008), pp. 560-568.
- Chandrasekar, M., Suresh, S., Bose, AC., Experimental investigations and theoretical determination of thermal conductivity and viscosity of Al2O3/water nanofluid, Exp. Therm. Fluid Sci., 34 (2010), pp. 210-216.
- ASHRAE Handbook, Fundamentals, American Society of Heating, Refrigerating and Air-Conditioning Engineers Inc., Atlanta, 1985.
- Kulkarni, DP., Das, DK., Vajjha, RS., Application of nanofluids in heating buildings and reducing pollution, Appl. Energy 86 (2009), pp. 2566-2573.
- Sundar, LS., Farooky, M.dH., Sarada, SN., Singh, MK., Experimental thermal conductivity of ethylene glycol and water mixture based low volume concentration of Al2O3 and CuO nanofluids, Int. Commun. Heat. Mass., 41 (2012), pp. 41-46.
- Yiamsawas, T., Mahian, O., Dalkilic, A.S., Kaewnai, S., Wongwises, S., Experimental studies on the viscosity of TiO2 and Al2O3 nanoparticles suspended in a mixture of ethylene glycol and water for high temperature applications, Appl. Energy 111 (2013), pp. 40-45.
- Yang, M.C., Scriven, L.E., Macosko, C.W., Some rheological measurements on magnetic iron-oxide suspensions in silicon oil, J. Rheo. 30 (1986), pp. 1015-1029.
- Odenbach, S., Stork, H., Shear dependence of field-induced contributions to the viscosity of magnetic fluids at low shear rates, J. Magn. Magn. Mater. 183 (1998), (1-2), pp. 188-194.
- Guo, S.Z., Li, Y., Jiang, J.S., Xie, H.Q., Nanofluids Containing γ-Fe2O3 Nanoparticles and Their Heat Transfer Enhancements, Nanoscale Res. Lett., 5 (2010), pp. 1222 - 1227.
- Abareshi, M., Sajjadi, S.H., Zebarjad, S.M., Goharshadi, E.K., Fabrication, characterization, and measurement of viscosity of α-Fe2O3 -glycerol nano fluids, J. Mol. Liq. 163 (2011), 1, pp. 27 - 32.
- Sundar, L.S., Ramana, E.V., Singh, M.K., De Sousa, A.C.M., Viscosity of low volume concentrations of magnetic Fe3O4 nanoparticles dispersed in ethylene glycol and water mixture, Chem. Phys. Lett. 554 (2012), pp. 236-242.
- Lee, S.W., Park, S.D., Kang, S., Bang, I.C., Kim, J.H., Investigation of viscosity and thermal conductivity of SiC nanofluids for heat transfer applications, Int. J. Heat Mass Trans. 54 (2011), pp. 433-438.
- Venerus, D.C., Buongiorno, J., Christianson, R., Townsend, J., I.C. Bang, et al., Viscosity Measurements on Colloidal Dispersions (Nanofluids) for Heat Transfer Applications, Appl. Rheol. 20 (2010) pp. 44582.
- Palabiyik, I., Witharana, S., Musina, Z., Ding, Y., Stability of glycol nanofluids - the consensus between theory and measurement, arXiv:1208.4207.
- Einstein, A., Investigations on the Theory of the Brownian movement, Dover Publications, New York, USA, 1956.
- Brinkman, H.C., The viscosity of concentrated suspensions and solutions, J. Chem. Phys., 20 (1952), pp. 571-581.
- Batchelor, G.K., Effect of Brownian-motion on bulk stress in a suspension of spherical-particles, J. fluid. Mech., 83 (1977), 1, pp. 97-117.
- Corcione, M., Empirical correlating equations for predicting the effective thermal conductivity and dynamic viscosity of nanofluids, Energy Conv. Manage., 52 (2011), pp. 789-793.